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Selective capture and separation of xenon and krypton using metal organic frameworks: a review

《化学科学与工程前沿（英文）》 2023年第17卷第12期页码 1895-1912 doi: 10.1007/s11705-023-2355-3

摘要： Xenon and krypton are widespread useful noble gases in commercial lighting, lasers, electronics, and medical industry. At the same time, radioactive noble gases may proliferate from used nuclear fuel and diffuse in open atmospheres. Metal organic frameworks as hotspot porous materials for gases uptake and separation are considered to be potential solutions. In this review, we comprehensively summarized recent researches on metal organic frameworks for selective capture and separation of xenon and krypton. Particularly, we followed the aspects of different optimal design strategies, including optimal pore/cage size and geometry, open metal sites, ions (anions and cations), and polar functional groups for enhancing the xenon adsorption and separation performances. Meanwhile, a comparison of each strategy and the mechanisms of xenon/krypton separation were pointed out. The separation of krypton from gases mixtures by dual-bed systems was further discussed. Finally, some existing challenges and opportunities for possible real applications were proclaimed.

关键词： metal organic frameworks xenon krypton selective separation used nuclear fuel

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中国新一代核能用材总体发展战略研究

干勇,赵宪庚,徐匡迪

《中国工程科学》 2019年第21卷第1期页码 1-5 doi: 10.15302/J-SSCAE-2019.01.001

摘要：

材料技术是支撑和保障核工程安全稳定运行的前提和基础。我国现有在役和在建的56台核电机组中有52台是压水堆，钠冷快堆和高温气冷堆正在开展示范工程电站的建设，其他堆型尚处于研究阶段。本文分析了我国新一代核能用材研发、制造、应用过程中存在的共性问题、在役和在建核能工程用材存在的突出问题、在研核能技术用材存在的关键问题，在此基础上提出了我国新一代核能用材的发展战略建议，包括设立国家新一代核能用材专业指导委员会，设立新一代核能用材国家专项基金或长期稳定支持的专项科技计划，创建我国新一代核能用材先进完整标准体系，建设国家层面的共享型工程级辐照实验装置，在独立自主原则下，继续开展新一代核能用材国际合作等。

关键词：新一代核能压水堆核能用材发展战略

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中国新一代核能核燃料总体发展战略研究

李冠兴,周邦新,肖岷,焦拥军,任忠鸣

《中国工程科学》 2019年第21卷第1期页码 6-11 doi: 10.15302/J-SSCAE-2019.01.002

摘要：

本文深入分析和研究了国内外压水堆燃料和材料技术，快堆及其他先进堆燃料技术以及核燃料循环相关材料技术发展的现状和趋势，提出了我国压水堆、快堆及其他先进堆核燃料与材料，以及核燃料循环材料发展的目标、发展路线图和重点任务。压水堆是我国21世纪相当长时间内核能发电及能源结构转型的主力堆型。作为压水堆发展重要支撑的核燃料及材料基本实现了国产化，但还没有实现品牌自主化。我国的快堆及快堆核燃料发展面临机遇和挑战，核燃料循环产业面临重大历史性发展机遇和巨大挑战。最后对我国的压水堆、快堆、其他先进堆型核燃料及材料，以及我国核燃料循环材料的发展提出了建议。

关键词：核燃料核材料轻水堆压水堆快堆燃料循环

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PWR-FBR with closed fuel cycle for a sustainable nuclear energy supply in China

XU Mi

《能源前沿（英文）》 2007年第1卷第2期页码 129-134 doi: 10.1007/s11708-007-0016-8

摘要： From the thermal reactor to the fast reactor and then to the fusion reactor; this is the three-step strategy that has been decided for a sustainable nuclear energy supply in China. As the main thermal reactor type, the commercialized development phase of the pressurized water reactor (PWR) has been stepped up. The development of the fast reactor (FBR) is still in the early stage, marked by China experimental fast reactor (CEFR), which is currently under construction. According to the strategy study on the fast reactor development in China, its engineering development will be divided into three steps: the CEFR with a power of 65 MWt/20 MWe; the China prototype fast reactor (CPFR) with a power of 1 500 MWt/600 MWe; and the China demonstration fast reactor (CDFR) with a power of 2 500 3 750 MWt/1 000 1 500 MWe. With regards to the fuel cycle, a 100 t/a PWR spent fuel reprocessing pilot plant and a 500 kg/ a MOX fabrication plant are under construction. A project involving the construction of an industrial reprocessing plant and an MOX fabrication plant are also under application phase.

关键词： reactor development reprocessing MWt/600 demonstration three-step strategy

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先进核燃料技术助推核能复兴

Mitch Leslie

《工程（英文）》 2021年第7卷第11期页码 1508-1510 doi: 10.1016/j.eng.2021.09.002

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核爆聚变电站──人类未来能源的希望

彭先觉,刘成安,陈银亮,郭勤,尹文华,白云,陈小伟,屈明

《中国工程科学》 2008年第10卷第1期页码 39-46

摘要：

详细介绍了核爆聚变电站的基本概念、组成、发展简史；提出了解决核爆炸实施安全、烧氘型核装置设计、核燃料生产回收等一系列问题的技术途径；对电站的技术可行性进行了分析论证，并比较了各种作为人类未来能源核能方案的前景。

关键词：核爆聚变电站爆洞喷钠烧氘型核装置核燃料循环

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我国核燃料循环标准化发展战略研究

潘建均,王毅韧,李筱珍,康椰熙,张宏伟,郭建新,郑刚阳,王妍妍

《中国工程科学》 2021年第23卷第3期页码 53-59 doi: 10.15302/J-SSCAE-2021.03.016

摘要：

核燃料循环标准化是核燃料循环产业安全发展、创新发展的重要支撑，特别是在我国进入高质量发展阶段期间，标准化作用显得尤为重要，开展核燃料循环标准化发展战略研究对支撑我国核工业强国建设具有重要战略意义。本文系统分析了国内外核燃料循环标准化的发展现状，从工作机制、发展平衡性、引领作用、保障能力等方面剖析了我国核燃料循环标准化亟待解决的关键问题，并据此提出了今后的主要任务和相关对策建议。研究指出，我国核燃料循环标准化工作今后的七项重点任务为：补齐核燃料循环后段标准短板、加大关键核心技术标准研制、加强先进标准研制、强化前沿基础标准建设、加强安全环保标准建设、深度参与国际标准化工作、强化标准化基础能力建设。最后，本文从将核燃料循环标准化纳入核工业“十四五”规划、健全标准化工作机制、加大经费投入、加强标准化人才队伍建设等方面提出了对策建议。

关键词：核燃料循环高质量发展技术标准基础能力标准国际化

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Evaluation of precipitation behavior of zirconium molybdate hydrate

Liang ZHANG, Masayuki TAKEUCHI, Tsutomu KOIZUMI, Izumi HIRASAWA

《化学科学与工程前沿（英文）》 2013年第7卷第1期页码 65-71 doi: 10.1007/s11705-013-1314-9

摘要： In the dissolution step of spent nuclear fuel, there is a world-concern problem that zirconium molybdate hydrate precipitates as a byproduct, and accumulates in some reprocessing equipments. In order to prevent this accumulation, we have developed a new method based on the controlled reaction crystallization of zirconium molybdate hydrate (ZMH) in the reprocessing solution, followed by solid liquid separation. In order to measure the particle size of ZMH, batch crystallization experiments were conducted by varying nitric acid concentration and operating temperature. In result, almost all particle sizes scatter around 1 μm on average, despite the higher concentration of nitric aid and operating temperature, and then small particles grow up as an aggregate sticking to the crystallizer. Moreover, polymorph and color changing were observed by varying the concentration of nitric acid and reaction time. These results suggest that crystal color and adhesiveness are closely related to the particle size of ZMH. And the control of nitric acid concentration and small particle growth would be the useful technique to prevent the ZMH sticking.

关键词： spent nuclear fuel zirconium molybdate hydrate cleaning method accumulation

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我国核电战略性新兴产业“十二五”培育与中长期发展展望

郭晴,苏罡

《中国工程科学》 2016年第18卷第4期页码 55-60 doi: 10.15302/J-SSCAE-2016.04.009

摘要：

核电技术产业是我国战略性新兴产业中新能源产业的重要构成部分，发展核电符合我国绿色低碳能源战略。按照科技突破引领产品升级，带动产能提升和产业发展的思路，本文系统地分析“十二五”期间核电技术产业培育和发展成果，重点介绍福岛事故后我国核电产业发展态势和“华龙一号”等先进核电技术的安全和经济特性，提出“十三五”乃至更长时期的发展趋势和方向，包括发展基于快堆的核燃料闭式循环体系，聚变技术发展实现“三步走”战略。通过小型模块化反应堆技术探索核能多用途利用等，实现核电技术产业的规模化、可持续发展，在推动我国经济平稳、持续增长，能源结构和工业结构优化升级方面发挥更大作用。

关键词：核电技术产业战略性新兴产业华龙一号核燃料闭式循环 “三步走”战略

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The origins of schedule management: the concepts used in planning, allocating, visualizing and managing

Lynda M. BOURNE, Patrick WEAVER

《工程管理前沿（英文）》 2018年第5卷第2期页码 150-166 doi: 10.15302/J-FEM-2018012

摘要： Getting the in the at the has always been a major organizational challenge. In ancient times this process seems to have been accomplished based on the scheme of arrangements being contained in the leader’s mind and instructions communicated verbally. Modern approaches to solving the twin challenges of first thinking through the ‘plan’ and then communicating the plan to the people who need to do ‘ ’ use sophisticated graphics, charts, diagrams, and computations. This paper traces the development of the concepts most project managers take for granted including bar charts and critical path schedules from their origins (which are far earlier than most people think) through to the modern day. The first section of the paper looks at the development of concepts that allow the visualization of time and other data. The second looks at the shift from static representations to dynamic modeling through the emergence of computers, dynamic calculations and integrated data from the 1950s to the present time.

关键词： time management scheduling CPM PERT Gantt Critical Path bar chart

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Second unmanipulated allogeneic transplantation could be used as a salvage option for patients with relapsed

《医学前沿（英文）》 2021年第15卷第5期页码 728-739 doi: 10.1007/s11684-021-0833-x

摘要： Relapse is the main problem after allogeneic hematopoietic stem cell transplantation (allo-HSCT). The outcome of a second allo-HSCT (HSCT2) for relapse post-HSCT has shown promising results in some previous studies. However, little is known about the efficacy of HSCT2 in patients with relapsed/refractory acute leukemia (AL) post-chemotherapy plus modified donor lymphocyte infusion (post-Chemo+m-DLI) after the first allo-HSCT (HSCT1). Therefore, we retrospectively analyzed the efficacy of HSCT2 in 28 patients with relapsed/refractory AL post-Chemo+m-DLI in our center. With a median follow-up of 918 (457–1732) days, 26 patients (92.9%) achieved complete remission, and 2 patients exhibited persistent disease. The probabilities of overall survival (OS) and disease-free survival (DFS) 1 year after HSCT2 were 25.0% and 21.4%, respectively. The cumulative incidences of nonrelapse mortality on day 100 and at 1 year post-HSCT2 were 7.1%±4.9% and 25.0%±8.4%. The cumulative incidences of relapse were 50.0%±9.8% and 53.5%±9.9% at 1 and 2 years post-HSCT2, respectively. Risk stratification prior to HSCT1 and percentage of blasts before HSCT2 were independent risk factors for OS post-HSCT2, and relapse within 6 months post-HSCT1 was an independent risk factor for DFS and relapse post-HSCT2. Our findings suggest that HSCT2 could be a salvage option for patients with relapsed AL post-Chemo+m-DLI.

关键词： second hematopoietic stem cell transplantation acute leukemia relapse chemotherapy modified donor lymphocyte infusion

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Kinematic, workspace and singularity analysis of a new parallel robot used in minimally invasive surgery

Alin STOICA, Doina PISLA, Szilaghyi ANDRAS, Bogdan GHERMAN, Bela-Zoltan GYURKA, Nicolae PLITEA

《机械工程前沿（英文）》 2013年第8卷第1期页码 70-79 doi: 10.1007/s11465-013-0365-4

摘要：

In the last ten years, due to development in robotic assisted surgery, the minimally invasive surgery has greatly changed. Until now, the vast majority of robots used in surgery, have serial structures. Due to the orientation parallel module, the structure is able to reduce the pressure exerted on the entrance point in the patient’s abdominal wall. The parallel robot can also handle both a laparoscope as well an active instrument for different surgical procedures. The advantage of this parallel structure is that the geometric model has been obtained through an analytical approach. The kinematic modelling of a new parallel architecture, the inverse and direct geometric model and the inverse and direct kinematic models for velocities and accelerations are being determined. The paper will demonstrate that with this parallel structure, one can obtain the necessary workspace required for a minimally invasive operation. The robot workspace was generated using the inverse geometric model. An in-depth study of different types of singularity is performed, allowing the development of safe control algorithms of the experimental model. Some kinematic simulation results and the experimental model of the robot are presented in the paper.

关键词： parallel robot minimally invasive surgery kinematics simulation

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Particle size distribution and shape control of Au nanoparticles used for particle gun

S. Kida, M. Ichiji, J. Watanabe, I. Hirasawa

《化学科学与工程前沿（英文）》 2013年第7卷第1期页码 60-64 doi: 10.1007/s11705-013-1313-x

摘要： Au nanoparticles are expected for the media to transfer genes into plants. However, the control of particle size distribution (PSD) and shape of Au nanoparticles is too difficult to design and prepare particles with suitable quality for the gene supporting media. Reduction crystallization experiments were performed in aqueous solution in order to clarify the effect of feeding conditions such as feeding profile, feeding rate, and feeding amount on PSD and shape of Au nanoparticles. Ascorbic acid (AsA) was selected as a reducing agent because it is safe for plants. Au particles of 50 nm, 50–200 nm, and 150–400 nm were obtained in batch operation, single-jet, and double-jet, respectively. Moreover, in single-jet and double-jet, the mean size of the obtained Au particles increases with the decrease of feeding rate or the increase of feeding amount. It is concluded that PSD of Au nanoparticles can be controlled in the range of 50–400 nm by changing feeding conditions of AsA and HAuCl aqueous solution.

关键词： reduction crystallization particle size distribution gene transferring media

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The electrostatic-alloy bonding technique used in MEMS

WANG Wei, CHEN Wei-ping

《机械工程前沿（英文）》 2006年第1卷第2期页码 238-241 doi: 10.1007/s11465-006-0011-5

摘要： Electrostatic-alloy bonding of silicon wafer with glass deposited by Au to form Si/Au-glass water, and bonding of Si/Au-glass with silicon wafer were researched during fabrication of pressure sensors. The silicon wafer and glass wafer with an Au film resistor were bonded by electrostatic bonding, and then Si-Au alloy bonding was formed by annealing at 400vH for 2 h. The air sealability of the cavity after bonding was finally tested using the N filling method. The results indicate that large bond strength was obtained at the bonding interface. This process was used in fabricating a pressure sensor with a sandwich structure. The results indicate that the sensor presented better performances and that the bonding techniques can be used in MEMS packaging.

关键词： Si/Au-glass strength MEMS packaging process sandwich structure

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Geosynthetics used to stabilize vegetated surfaces for environmental sustainability in civil engineering

Jie HAN,Jun GUO

《结构与土木工程前沿（英文）》 2017年第11卷第1期页码 56-65 doi: 10.1007/s11709-016-0380-8

摘要： Geosynthetics, factory-manufactured polymer materials, have been successfully used to solve many geotechnical problems in civil engineering. Two common applications are earth stabilization and erosion control. Geosynthetics used for earth stabilization include but are not limited to stabilized slopes, walls, embankments, and roads. Geosynthetics used for erosion control are mostly related to slopes, river channels and banks, and pond spillways. To enhance environmental sustainability, vegetation has been increasingly planted on the facing or surfaces of these earth structures. Under such a condition, geosynthetics mainly function as surficial soil stabilization while vegetation provides green appearance and erosion protection of earth surfaces. Recently, geosynthetic or geosynthetic-like material has been used to form green walls outside or inside buildings to enhance sustainability. Geosynthetics and vegetation are often integrated to provide combined benefits. The interaction between geosynthetics and vegetation is important for the sustainability of the earth and building wall surfaces. This paper provides a review of the current practice and research in the geosynthetic stabilization of vegetated earth and building surfaces for environmental sustainability in civil engineering with the emphases on geosynthetic used for erosion protection, geosynthetic-stabilized slopes, geosynthetic-stabilized unpaved shoulders and parking lots, and geosynthetic-stabilized vegetated building surfaces.

关键词： erosion geosynthetic stabilization sustainability vegetation